Abstract
Two-dimensional electronic spectroscopy (2DES) allows fundamentally new insights into the structure and dynamics of multi-chromophore systems. So far two schemes have been successfully used to implement 2DES in the visible range: the heterodyne detected three-pulse photon echo [1] and the partially collinear pump-probe geometry [2]. The latter employs two phase-locked collinear pump pulses and a non-collinear probe pulse which is dispersed on a spectrometer. Advantages of this configuration are its simplicity, its applicability to standard pump-probe systems and the fact that it automatically measures absorptive spectra.
© 2013 IEEE
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