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Electronic Coherence Mediated Quantum Control of Chemical Reactions in Polyatomic Molecules

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Abstract

We report order-of-magnitude quantum coherent control of the yield of photofragment ions following the creation of electronic coherence in the Rydberg states of dicyclopentadiene (C10H12) molecules using a pair of phase-locked femtosecond near-infrared laser pulses.

© 2013 Optical Society of America

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