Observing the Interplay Between Surface and Bulk Optical Nonlinearities in Thin Van Der Waals Crystals

Skylar Deckoff-Jones; Jingjing Zhang; Christopher E. Petoukhoff; Michael K.L. Man; Sidong Lei; Robert Vajtai; Pulickel M. Ajayan; Diyar Talbayev; Julien Madéo; Keshav M. Dani

doi:10.1364/CLEO_QELS.2016.FTu1A.7

Conference on Lasers and Electro-Optics
OSA Technical Digest (online) (Optica Publishing Group, 2016),
paper FTu1A.7
•https://doi.org/10.1364/CLEO_QELS.2016.FTu1A.7

Observing the Interplay Between Surface and Bulk Optical Nonlinearities in Thin Van Der Waals Crystals

Skylar Deckoff-Jones, Jingjing Zhang, Christopher E. Petoukhoff, Michael K.L. Man, Sidong Lei, Robert Vajtai, Pulickel M. Ajayan, Diyar Talbayev, Julien Madéo, and Keshav M. Dani

CLEO: QELS_Fundamental Science 2016

San Jose, California United States
5–10 June 2016
ISBN: 978-1-943580-11-8

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Novel Optical Materials (FTu1A)

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S. Deckoff-Jones, J. Zhang, C. E. Petoukhoff, M. K. L. Man, S. Lei, R. Vajtai, P. M. Ajayan, D. Talbayev, J. Madéo, and K. M. Dani, "Observing the Interplay Between Surface and Bulk Optical Nonlinearities in Thin Van Der Waals Crystals," in Conference on Lasers and Electro-Optics, OSA Technical Digest (online) (Optica Publishing Group, 2016), paper FTu1A.7.

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Abstract

Thickness dependence of second harmonic generation in atomically thin InSe is studied. A strong resonance is observed, attributed to interference between distinct surface and bulk nonlinear contributions.

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