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Single Molecular Vibrational Relaxation Dynamics and Adsorbate Fluctionality

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Abstract

Tip-enhanced Raman spectroscopy at cryogenic temperatures probes the intrinsic linewidths of vibrational modes. Temperature dependent investigation of small ensembles reveals ultrafast vibrational relaxation dynamics, conformational heterogeneity, and single molecule fluctionality on the time scale of seconds.

© 2015 Optical Society of America

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