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Ultrafast recovery of valence electrons in 1,3-butadiene probed by time-resolved photoelectron spectroscopy with high harmonic pulses

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Abstract

Ultrafast recovery of the valence electrons to the ground state in 1,3-butadiene with time constants of 53~99 fs after photoexcitation was observed by time-resolved photoelectron spectroscopy using high harmonic pulses for the first time.

© 2013 Optical Society of America

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