Physical Origins of Strong Chiral Sensitivity of High Harmonic Generation

R. Cireasa; A. E. Boguslavskiy; A. E. Boguslavskiy; A. E. Boguslavskiy; B. Pons; M. C. H. Wong; D. Descamps; S. Petit; H. Ruf; N. Thire; N. Thire; A. Ferre; J. Suarez; J. Higuet; B. E. Schmidt; A. F. Alharbi; F. Legare; V. Blanchet; V. Blanchet; B. Fabre; S. Patchkovskii; S. Patchkovskii; O. Smirnova; Y. Mairesse; V. R. Bhardwaj

2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference
(Optica Publishing Group, 2015),
paper CG_6_2

Physical Origins of Strong Chiral Sensitivity of High Harmonic Generation

R. Cireasa, A. E. Boguslavskiy, B. Pons, M. C. H. Wong, D. Descamps, S. Petit, H. Ruf, N. Thire, A. Ferre, J. Suarez, J. Higuet, B. E. Schmidt, A. F. Alharbi, F. Legare, V. Blanchet, B. Fabre, S. Patchkovskii, O. Smirnova, Y. Mairesse, and V. R. Bhardwaj

The European Conference on Lasers and Electro-Optics 2015

Munich Germany
21–25 June 2015
ISBN: 978-1-4673-7475-0

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Sub-fs Dynamics in Molecules (CG_6)

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R. Cireasa, A. E. Boguslavskiy, B. Pons, M. C. H. Wong, D. Descamps, S. Petit, H. Ruf, N. Thire, A. Ferre, J. Suarez, J. Higuet, B. E. Schmidt, A. F. Alharbi, F. Legare, V. Blanchet, B. Fabre, S. Patchkovskii, O. Smirnova, Y. Mairesse, and V. R. Bhardwaj, "Physical Origins of Strong Chiral Sensitivity of High Harmonic Generation," in 2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference, (Optica Publishing Group, 2015), paper CG_6_2.

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Abstract

We demonstrate extreme chiral sensitivity of high harmonic generation from randomly oriented ensemble of chiral molecules in elliptical mid-infrared fields, and explain the physical mechanism underlying this very strong, highly nonlinear chiro-optical response. We also use the high harmonic spectra to resolve the electronic chiral response with 0.1 femtosecond temporal resolution.

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