Abstract
High-order harmonic generation (HHG) from nonadiabatically aligned molecules [1,2] provides an effective tool for studying structures and dynamics of gas phase molecules, where the angle-dependent harmonic yield around the molecular axis is the key to deduce the characteristic properties of a single molecule. The harmonic distribution observed in the HHG experiment, however, always includes some broadening of the molecular axis distribution that blurs the shape of a single molecule, due to the imperfect alignment of molecules.
© 2011 Optical Society of America
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