Abstract
The strength of stimulated Brillouin scattering (SBS) in optical fibers is largely governed by the spatial overlap between supported optical and acoustic modes, leading to a complicated amalgamation of photon-phonon interactions in multimode fibers. Here, we study SBS dynamics in ring-core fibers that support modes carrying orbital angular momentum (OAM), which result in distinctive characteristics. We find that the OAM SBS response, as well as modal content, strongly depends on the polarization state of the pump, as OAM modes in fiber have distinct propagation dynamics depending on whether the input is circularly or linearly polarized. This is in contrast to conventionally posited wisdom that SBS strength is independent of the pump’s input polarization state in an isotropic material. This increased specificity can lead to interesting effects such as spatial phase conjugation even in the presence of stably transmitted, i.e. non-aberrated, spatial pump modes. More generally, we show that using OAM modes yields additional degrees of control over SBS interactions beyond more conventional parameters, such as effective area, acousto-optic spatial overlaps, and material composition.
© 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
Stimulated Brillouin scattering (SBS) is an important acousto-optic nonlinearity in optical fibers that has led to a variety of applications [1], including distributed sensing [2], light amplification [3], and slow light generation [4]. SBS is also a debilitating phenomenon that can act as a limitation for high powered fiber lasers [5,6] or impact long-haul communication systems [7,8]. As such, there is a desire to suppress SBS, or at least make it more controllable, which so far has been achieved mainly through waveguide design that changes the interactions between light and sound or by spectrally broadening the pump source [9,10]. SBS is also well known as one of the easiest and most reliable ways of producing phase conjugation [11], which is of interest for uses in aberration correction [12,13], optical trapping [14], and signal processing [15]. SBS has been extensively studied for conventional eigenmodes in multimode fibers [16–19]. But since modes in an optical fiber can also be expressed in terms of the orbital angular momentum (OAM) and spin angular momentum (SAM) they carry, SBS can also be analyzed in this modal basis. Here, we show that fibers stably guiding a large ensemble of high order OAM modes yield new forms of control over the SBS process due to modified mode selection rules and phase matching criteria, which also leads to the spontaneous generation of record high order OAM acoustic waves.
The OAM carried by optical fiber modes is quantified by a topological charge $ \pm \mathrm{{\cal L}}$ that represents the directional twisting of the helical phase front per wavelength [20]. The SAM carried by these fiber modes is represented by its left or right circular polarization state, ${\hat{\sigma }^ \pm }$, respectively. Confined by a fiber in which they stably propagate [21], these supported ${\pm} \mathrm{{\cal L}; {\hat{\sigma }^ \pm }}$ modes experience a spin-orbit interaction (SOI), which makes the propagation constant of the mode dependent on the chirality, or sign, associated with both their OAM and SAM. This SOI dependence on chirality leads to the emergence of circular birefringence in an otherwise circularly symmetric, isotropic fiber, which changes the propagation constant of the left and right handed circularly polarized SAM states. Hence, linearly polarized light of given OAM, when introduced into these fibers, experiences optical activity (OA) [22] – i.e., linear polarization rotation with propagation, which mimics a property that has been traditionally associated with anisotropic chiral materials. We have found that this attribute – of distinct propagation behavior arising from SOI-induced chirality – plays a significant role in changing the dynamics of SBS of these fiber modes. In the case of circularly polarized OAM-carrying pumps ${\pm} \mathrm{{\cal L}; {\hat{\sigma }^ \pm }}$, highly multimoded Stokes is observed, whose modal content is dictated by spatial overlap integrals (in analogy to the observed behavior from conventional fiber modes in standard fibers) and angular momentum conservation. In contrast, linearly polarized OAM pumps $\mathrm{{\cal L} };\hat{x}$ that experience OA exhibit dramatically different SBS modal behavior. Specifically, we see the rotational evolution of the polarization forces all Stokes light into a spatially phase conjugated state, suppressing other SBS interactions. We demonstrate how the SBS behaviors for each polarization state, circular and linear, differ from one another, in stark contrast to SBS behavior in conventional fibers, where it is agnostic to pump polarization state [23]. This suggests that the OAM content of light represents an attractive toolbox with which to control SBS nonlinear interactions in optical fibers.
2. OAM propagation dynamics in fibers
The ring-core optical fibers in which we conduct our studies are designed to support a large count of mode-mixing-free, stable OAM optical modes ($|\mathrm{{\cal L}} |> 20$ at 1 µm wavelengths), hence yielding a highly multimoded platform in which to study SBS [24]. The fiber is an isotropic and circularly symmetric medium, which is shown by the image of the fiber facet in Fig. 1(a). To differentiate fiber modes, we consider the chirality, or sign, of $\mathrm{{\cal L}}$ and $\hat{\sigma }$. If these two quantities match in sign, then the fiber mode is a spin-orbit aligned (SOa) mode, and if they are opposite, it is a spin-orbit anti-aligned (SOaa) mode. Their electric fields are given by:
3. OAM SBS responses and setup
SBS gain g, in optical fibers can be characterized by an acousto-optic effective area $A_{eff}^{ao}$ [1]. In spatial modes that carry OAM and SAM, angular momentum must also be conserved, a principle that has been demonstrated in previous works [28–30]. Heterodyne measurements along with waveguide eigenvalue calculations (measurements, matching calculations within 1.23%, are described later in section 4.2) affirm that the SBS we observe is a result of dominating axial-strain / longitudinal displacement acoustic modes ${u_z}$, which are described with complex envelope $\tilde{\rho }({z,t} )$, acoustic frequency $\mathrm{\Omega }$, and propagation constant q [1].
As we can see from Eq. (3), these acoustic phonons can carry the OAM helical phase with charge $\mathrm{{\cal L}}$, but since they are longitudinally polarized, they cannot carry SAM. This means that SAM conservation is satisfied only between the pump and Stokes optical fields, while OAM conservation is achieved through the interplay of all participating optical and acoustic modes. For a pump with OAM ${\mathrm{{\cal L}}_{pump}}$ and Stokes in a spatial mode with OAM ${\mathrm{{\cal L}}_{stokes}}$, the well-known expression for acousto-optic effective area can be written in a modified form of [1,31]:
Another interesting observation is that the blue and red curves in Fig. 2(c) never cross. This indicates that the allowed SBS processes never produce an optimally overlapped acousto-optic interaction and there is always some spatial walk-off present between the optical and acoustic modes. This points to the proclivity of OAM conservation to reduce the SBS Stokes’ gain. Focusing now on the phase conjugated ${\mathrm{{\cal L}}_{stokes}} = {\mathrm{{\cal L}}_{pump}} = 30$ interaction, we find that there are 14 other SBS interactions (${\mathrm{{\cal L}}_{stokes}} = 19$ to $33$) with comparable $A_{eff}^{ao}\sim{\pm} 1\; \textrm{dB}$, showing that many of these processes have similar strengths despite spanning a wide modal range. The fact that many of these SBS interactions have such similar acousto-optic effective areas is attributed to the near identical ring field profiles shared by OAM modes, which we presented in Fig. 1(c) (these strong spatial similarities of OAM modes are especially evident when compared to other modes supported in multimode fibers [32]). As such, we expect that, for a circularly polarized OAM pump, the generated Stokes light will be partitioned into a multitude of higher order modes. And, as we will see later, linearly polarized pumps experiencing chiral OA have an additional constraint that restricts the modes in which the Stokes occurs.
Our setup to test SBS with OAM modes is illustrated in Fig. 3(a). It uses a pump laser at 1045 nm that produces rectangular 1-μs pulses at a 5 kHz rep-rate with peak power exceeding 100 W (see Fig. 3(b)). To launch the forward-propagating OAM pump modes of interest into our 50-m ring-core fiber, the beam from our laser source is spatially sculpted with a spatial light modulator (SLM1) to impart it with topological charge ${\mathrm{{\cal L}}_{pump}}$, while a rotating quarter wave plate (QWP) is used to set the polarization state as either circular ${\hat{\sigma }^ - }$ or linear $\hat{x}$. We ensure that this combination of pulse length and fiber length would allow us to treat the SBS response as if the pump were effectively a continuous-wave source, while avoiding any transient effects [33]. Additionally, for each ${\mathrm{{\cal L}}_{pump}}$ mode that is used in our experiments pump power, ${P_{pump}}(\mathrm{{\cal L}} )$, is adjusted to compensate for the respective change in modal launch loss into the fiber, ensuring that all SBS responses are tested with effectively the same pump power. The injected pump peak powers into the fiber are ${P_{pump}}({24} )= 29.3\; \textrm{W}$, ${P_{pump}}({26} )= 32.2\; \textrm{W}$, ${P_{pump}}({28} )= 32\; \textrm{W}$, and ${P_{pump}}({30} )= 35\; \textrm{W}$. This is done by using a half wave plate (HWP1) and polarization beam splitter (PBS) to change the amount of $\hat{x}$ light incident on the polarization selective SLM. With these pump powers, we conduct our measurements above threshold power [1], i.e. in the high gain (strong scattering) regime [34]. The output of the fiber is imaged onto a CCD camera to perform mode purity analysis with spatial interferometry techniques [35], which verify >20 dB mode excitation purities, with polarization extinction ratios measured to be >15 dB. This means the pump is monomoded despite the fiber being multimoded. The back-scattered Stokes is redirected with a beam splitter (BS) to a mode sorter comprising another SLM2 (which applies an additional topological charge of ${\mathrm{{\cal L}}_{mode - sorter}}$) and single mode fiber (SMF), which when sent to an optical spectrum analyzer (OSA), allows measuring modal power of the Stokes with extinction ratios >20 dB [24]. This mode sorting technique is also capable of separating Rayleigh back-reflected light from the SBS Stokes. Since Rayleigh scattered light exists exclusively in the $- {\mathrm{{\cal L}}_{pump}}$ mode, any applied ${\mathrm{{\cal L}}_{mode - sorter}}$ that does not specifically select for it will transform the Rayleigh light into a ${\mathrm{{\cal L}}_{pump}} + {\mathrm{{\cal L}}_{mode - sorter}}$ OAM mode that does not couple into the SMF, effectively filtering it out. The power and absolute spectrum (10 pm resolution) of each sorted ${\mathrm{{\cal L}}_{stokes}}$ mode is then measured with the OSA, and its RF spectrum is obtained by performing heterodyne measurements (orange shaded box in Fig. 3(a)) [36]. The heterodyne beat frequency between the pump and Stokes is measured with an electronic spectrum analyzer (ESA), which enables relative spectral measurements of the acoustic frequency and linewidth from each ${\mathrm{{\cal L}}_{stokes}}$ spectrum with 10 kHz resolution. For the OA $\mathrm{{\cal L}};\hat{x}$ pump case, Stokes measurements are determined by combining OSA and ESA measurements taken at two orthogonal polarizations for each ${\mathrm{{\cal L}}_{stokes}}$ sorted mode.
4. OAM SBS results
4.1 Stokes power measurements
First, we examine SBS dynamics utilizing circularly polarized SOaa ${\mathrm{{\cal L}}_{pump}};$ $\hat{\sigma}^{-}$modes as our pump. As an example, we use a pump mode with ${\mathrm{{\cal L}}_{pump}} = 28$, while the mode sorter is set to ${\mathrm{{\cal L}}_{mode - sorter}} ={-} 28$. If the Stokes beam were comprised of only a single specific mode, the mode sorter would convert the back-scattered beam into a distinctive Bessel-beam pattern (in the far-field). Instead, as shown in Fig. 4(a), a massively multimoded beam is recorded (at first glance, it may appear Gaussian in shape, but we experimentally confirm it to resemble a speckle pattern comprising many modes). Quantifying this with OSA measurements (Fig. 4(b)) shows that the Stokes power in the representative modes ${\mathrm{{\cal L}}_{stokes}} = [{22, 28, 33} ]$ are similar, confirming the multimoded nature of the Stokes light, as deduced from the image of Fig. 4(a). We repeat these measurements with different pump modes, and summarize our findings in Fig. 4(c). The Stokes manifests over a broad range of backward propagating modes regardless of the topological charge of the pump. The mode with the highest Stokes power (yellow stars in Fig. 4(c)) shifts to increasingly higher order OAM modes, with exception of the ${\mathrm{{\cal L}}_{pump}} = 30$ mode, where it appears to occur for a lower order mode. This drop in power for the $\mathrm{{\cal L}} \ge 30$ modes is not a result of lower spatial overlaps from Eq. (4), but is instead due to the fact that the $\mathrm{{\cal L}} \ge 30$ modes in our fiber are approaching cutoff and possess larger linear propagation losses [37]. We also observed negligible amounts of Stokes power in modes with ${\mathrm{{\cal L}}_{stokes}}$ of opposite sign as ${\mathrm{{\cal L}}_{pump}}$ – i.e. the reflected modes that would have interacted only with acoustic modes of low topological charges ${\mathrm{{\cal L}}_A}$. We again note that Rayleigh reflected light in the $- {\mathrm{{\cal L}}_{pump}}$ mode has been filtered out from the SBS Stokes power measurements as a result of us using our mode sorter to select for only $+ |\mathrm{{\cal L}} |$ modes. Hence, to summarize, SBS arising from pump modes that carry a well-defined OAM in a circular polarization state scatters light into a multitude of OAM Stokes modes that are generally close to ${\mathrm{{\cal L}}_{pump}}$ while strongly preferring interactions involving very high acoustic OAM.
For the second round of measurements, we turn our attention to linearly polarized OA $\hat{x}$ states as our pump. Portrayed in Fig. 4(d) is the far-field Stokes image formed from a ${\mathrm{{\cal L}}_{pump}} = 28$ and with the mode sorter set to ${\mathrm{{\cal L}}_{mode - sorter}} ={-} 28$, as before. In sharp contrast to Fig. 4(a), the image now depicts a clear Bessel-beam-like pattern, suggesting that the Stokes has been substantially generated in the ${\mathrm{{\cal L}}_{stokes}} = 28$ mode alone. Quantitative power measurements with the OSA conducted at one HWP position (Fig. 4(e)) show that the Stokes power in modes with ${\mathrm{{\cal L}}_{stokes}}$ adjacent to the phase conjugated state are nearly extinguished (note that this Fig. shows mode extinction of ∼20 dB, which corresponds to the noise-floor of this measurement technique). The power matrix in Fig. 4(f) demonstrates a universal principle for linearly polarized pumps. The entirety of the produced Stokes power appears to exist only in the same $\mathrm{{\cal L}}$ mode order as the pump, while the power in all other measured modes reside at the mode sorter noise floor. Note, as mentioned above, that we quantitatively measured Stokes power in only the adjacent mode orders – for mode orders further than ${\mathrm{{\cal L}}_{pump}} \pm 2$, a full quantitative analysis was unnecessary since we qualitatively confirmed that negligible power existed in them.
4.2 Heterodyne measurements
To further study the OAM SBS behavior of the acoustic vortices supported in our fiber, we conducted heterodyne measurements with the setup shown in Fig. 3(a). Figure 5(a) shows an ESA trace of the Stokes spectrum (blue), with an applied functional fit (red), generated from a ${\mathrm{{\cal L}}_A} = 52$ acoustic phonon with circularly polarized ${\mathrm{{\cal L}}_{pump}} = 26$ and ${\mathrm{{\cal L}}_{stokes}} = 26$ modes. Since we are operating above threshold power, gain-narrowing effects validates the use of a Gaussian fit [34]. From this curve fitting we measure the Brillouin frequency and spectral linewidth of each ${\mathrm{{\cal L}}_A}$ phonon. Figure 5(b) shows the acoustic frequencies for the different phonons, produced from various acousto-optic interactions over the modal space (sorted by which ${\mathrm{{\cal L}}_{pump}}$ was used). Although all acoustic frequencies are measured to be around ∼14 GHz, they are unique for each combination of participating [${\mathrm{{\cal L}}_{pump}}$; ${\mathrm{{\cal L}}_{stokes}}$] optical fields. For example, the ${\mathrm{{\cal L}}_A} = 54$ acoustic phonons associated with the [${\mathrm{{\cal L}}_{pump}} = 24;$ ${\mathrm{{\cal L}}_{stokes}} = 30$] and [${\mathrm{{\cal L}}_{pump}} = 30;$ ${\mathrm{{\cal L}}_{stokes}} = 24$] interactions have the same frequency (green-dashed circle), but this is different from the ${\mathrm{{\cal L}}_A} = 54$ phonons associated with the [${\mathrm{{\cal L}}_{pump}} = 26;$ ${\mathrm{{\cal L}}_{stokes}} = 28$] and [${\mathrm{{\cal L}}_{pump}} = 28;$ ${\mathrm{{\cal L}}_{stokes}} = 26$] interactions (which themselves have nearly the same measured frequencies, pink-dashed circle). We also performed these measurements using optically active linearly polarized pumps, specifically probing the OA phase conjugated acousto-optic interactions (black x’s in Fig. 5(b)). Here we find that acoustic frequency is independent of the state of polarization used, as we see in the blue-dashed oval, where circularly and linearly polarized [${\mathrm{{\cal L}}_{pump}} = 24;$ ${\mathrm{{\cal L}}_{stokes}} = 24$] interactions produce acoustic phonons with very similar frequencies. This indicates that acoustic frequency is governed by the traditional SBS phase matching conditions between optical and acoustic modes [1]. Next, Fig. 5(c) shows the linewidth measurements of each phonon associated with the combinations of circularly polarized ${\mathrm{{\cal L}}_{pump}}$ and ${\mathrm{{\cal L}}_{stokes}}$ modes, as distinguished by the measured frequencies from Fig. 5(b). All linewidths are found to all be approximately 20 MHz (with the exception of certain Stokes modes generated from ${\mathrm{{\cal L}}_{pump}} = 24$), which suggests that our phonons are indeed experiencing gain-narrowing [34]. Therefore, although the previous section showed distinctive mode-selection and polarization dependencies for OAM carrying pumps, the associated acoustic frequencies and linewidths follow the well-established phase matching rules and dynamics for SBS in standard multimode fibers.
5. Discussion
The SBS measurements described in section 4 can be summarized as follows. When the pump is in a circular polarization state, carrying a well-defined topological charge ${\mathrm{{\cal L}}_{pump}}$, backward propagating Stokes light scatters into a multitude of modes with topological charge close to the value of ${\mathrm{{\cal L}}_{pump}}$. The highest power Stokes mode also appeared to prefer shifting towards higher mode orders, though this trend was seen to break down for ${\mathrm{{\cal L}}_{pump}} = 30$, but, as we noted previously, that is simply because modes of $\mathrm{{\cal L}} \ge 30$ become quite lossy in our fiber [37]. The reason for this is that the SBS process strongly prefers modes with ${\mathrm{{\cal L}}_{stokes}}$ that is of the same sign and near the absolute value as that of ${\mathrm{{\cal L}}_{pump}}$ – i.e. modes that have undergone a mode transformation mediated by very high order acoustic modes with ${\mathrm{{\cal L}}_A} \approx 2 \cdot {\mathrm{{\cal L}}_{pump}}$ – in accordance with the OAM conservation mode selection rule. It is interesting to note that the system naturally prefers to generate high OAM acoustic modes (as high as $63$ in our experiments) in contrast to conventional SBS in standard fibers, which typically do not generate, or at least prefer, high OAM sound vibrations. But given Eq. (4), Fig. 2, and the discussion in section 3, this is not unexpected. The SBS process always chooses the mode combinations that result in high overlap integrals, and for high OAM charge pumps, these overlaps turn out to simply be with acoustic modes with roughly double the twist rates.
The SBS behavior observed with linearly polarized pumps carrying OAM is markedly different. These (pump) modes obviously have the same field amplitude profiles as circularly polarized modes, which may appear to imply that Eq. (4) and all the discussion from section 3 should predict similar behavior of that observed when the pump is circularly polarized, especially since conventional SBS theory posits that its strength (and hence dynamics) is identical regardless of the polarization state of the pump [23]. Instead, we find that the Stokes light occurs in only one mode, which is strictly phase conjugated with respect to the pump. We note that the SBS phase conjugation presented here is produced by stably propagating beams with no mode scrambling, whereas conventional multimode fibers typically experience SBS phase conjugation primarily with aberrated, or speckled, pumps [13,38]. The explanation of this peculiar behavior lies in the fact that a linearly polarized fiber OAM mode is not a single eigenmode, but rather a superposition of two, namely the SOa and SOaa $+ \mathrm{{\cal L}};{\hat{\sigma }^ \pm }$ modes described in section 2. This linear polarization yields optical activity – i.e., a stable rotation of the modes’ polarization as it propagates, mimicking a chiral material, as illustrated in Fig. 1(e) and described by Eq. (2). Hence, Eq. (4) is no longer sufficient to characterize this interaction, and we need to additionally invoke the nonlinear photon-phonon amplitude differential equations [23,39], such as $\partial {A_{si}}/\partial z \propto {g_m}{\tilde{\rho }^*}{A_{pi}}$, which specifically describes an interaction of light in a pump mode, $p = pump$, scattering from an acoustic phonon into a Stokes mode, $s = stokes$. Since the optically active states of the pump and Stokes represent a total of four distinct optical fields, each with two distinct orthogonal polarizations, these differential equations have two components – one where all interacting fields are of the same polarization – the conventional case in single-polarization interactions (already discussed in section 3), and one where they are pair-wise orthogonal, yielding cross-modal SBS interactions. This latter contribution to SBS, relevant for the optically active states, can be represented as:
There is a more intuitive explanation for the emergence of the aforementioned phase matching condition for SBS with OAM fiber modes. Recall, from section 2 (see, especially, Fig. 1(e)) that an OA state possesses a unique chiral attribute wherein its amplitude remains constant during fiber propagation but its linear polarization state systematically rotates. The rotation rate is a strong function of topological charge, or OAM content $\mathrm{{\cal L}}$. Since SBS is highly polarization-selective [1], the SBS interaction that remains non-negligible is the phase conjugated ${\mathrm{{\cal L}}_{stokes}} = {\mathrm{{\cal L}}_{pump}}$ interaction because this is the only mode that mimics, i.e. retraces, the polarization evolution of the pump (see Fig. 6(c)). However, for all other counter-propagating modes with ${\mathrm{{\cal L}}_{stokes}} \ne {\mathrm{{\cal L}}_{pump}}$, with Stokes in OAM topological charge of the same (Fig. 6(d)) or opposite (Fig. 6(e)) sign, the rotational behaviors of the pump and Stokes quickly drift apart, resulting in polarization walk-off and low nonlinear gain. Since this rotation rate is intimately tied to the phase difference between the SOa and SOaa modes whose superposition is a linear polarization state, Stokes produced from pumps in OA states depends on an engineered phase matching relationship in an otherwise self-phase matched SBS process. This illustrates a new mechanism of control over SBS with OA: polarization overlap. Since the phase conjugated interaction maximizes the polarization overlap, it is a highly preferred process and receives significant cross-modal photon-phonon gain (see Eq. (5)). Whether one uses the photon-phonon nonlinear amplitude equations or polarization rotational overlap, it is evident that SOI-induced propagation constant splitting in OAM carrying fibers plays a critical role in determining the spatial modes in which substantial SBS gain can be obtained, in sharp contrast to SBS behavior in conventional multimode fibers with standard (i.e. zero-OAM, so-called, LP) modes.
6. Conclusion
To summarize, the work we present here examines the dynamics of SBS that arise from using a fiber that stably supports a large ensemble of OAM carrying modes. For instance, a simple change in the input polarization state of the pump diverts Stokes-scattered light from occupying several back-propagating modal states to a single phase conjugated state. In contrast, the strength of SBS responses are conventionally considered to be insensitive to the polarization state of the pump. Moreover, while spatial phase conjugation has long been known to occur for SBS, this is primarily in the context of an aberrated pump beam, whereas our experiments used stably propagating modes. This distinctive behavior arises from an inherent chirality induced by linearly polarized light carrying OAM in optical fibers, which introduced a novel, engineerable phase matching criterion, in an otherwise self-phase-matched (SBS) process. OAM conservation laws also imply that the Stokes generated in these fibers are mediated by acoustic modes of record high OAM (${\mathrm{{\cal L}}_A} = 63$) – in fact, the overlap integrals require that the spontaneously generated sound waves due to OAM carrying pumps carry roughly twice the topological charge of the optical modes. In general, we show that the angular momentum content of light plays a critical role in controlling the strength, modal content and frequency of the Stokes light, and hence represents an alternative toolbox with which SBS can be controlled in optical fibers.
Funding
Vannevar Bush Faculty Fellowship (N00014-19-1-2632); Multidisciplinary University Research Initiative (N00014-20-1-2450); Air Force Office of Scientific Research (FA9550-14-1-0165).
Acknowledgments
The authors would like to thank X. Liu and H.B. Kabagöz for their insightful discussions, and A. McCall for his instrumentation work.
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
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