Abstract
The transverse nature of light leads to longitudinal optical spin. Here, the unprecedented transverse optical spin of propagating waves and guided modes in a gyroelectric medium is clarified. We identify the propagation modes in a bulk gyroelectric medium and their polarization in terms of optical spin. The anisotropic permittivity of a gyroelectric medium results in two propagation modes, slow and fast, in which the optical spin varies according to the propagation direction. When the magnetization direction of the gyroelectric medium and the propagation direction of the light are not parallel, these modes possess both the longitudinal and transverse components of optical spin. We also confirm that a gyroelectric slab waveguide induces transverse optical spin in the guided light. We investigate the transport behavior of transverse optical spin in a gyroelectric slab using numerical calculations with a modified 3D finite difference time domain method. These new gyroelectric guided modes offer a novel approach to the manipulation of optical spin on a nanoscale.
© 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
1. Introduction
The exchange of spin angular momentum between light and matter has attracted significant research interest for its potentially wide range of applications [1,2]. Chiral light–matter interaction has been actively investigated in the study of chiral molecules and spin-polarized quantum emitters, which has opened new research avenues such as chiral sensing [3–6] and chiral spin–photon interfaces [7–10]. Unlike light waves in free space, manipulating optical spin in a confined geometry is a challenge because polarization is predetermined by the boundary conditions of photonic structures. Many optical waveguides or cavity structures, due to their symmetry, support only linearly polarized transverse electric (TE) or transverse magnetic (TM) modes with zero net optical spin.
It has recently been pointed out that any evanescence field of confined light possesses transverse optical spin [11,12]. In addition, the transverse surface conductivity of graphene is known to support chiral plasmon polaritons at its edge [13,14]. Evanescence fields and chiral plasmon polaritons are related to edge states that exhibit spin-momentum locking. This one-to-one relationship between the handedness of the optical spin and the propagation direction of the light enables chiral light–matter interaction to be investigated [15,16]. However, the net optical spin averaged over the entire evanescent regions of a waveguide is zero if the symmetry of the structure is not broken. In considering transverse optical spin as a potential unit of information, it is highly desirable to find a propagating mode that intrinsically carries non-zero net optical spin regardless of the propagation direction of the light.
Here, we present a novel propagating or guided mode that carries intrinsic optical spin. We consider a medium with gyroelectric permittivity and show that the transverse optical spin of propagating waves arises in this gyroelectric medium. We identify the presence of fundamental slow and fast modes in the system and investigate their optical properties. Remarkably, we find that transverse optical spin exists for both the slow and fast modes when the magnetization direction of a gyroelectric medium and the propagation direction of the light are not parallel. We also suggest that even a confined mode in a gyroelectric slab waveguide possesses transverse optical spin. Using a modified 3D finite difference time domain (FDTD) method with the permittivity tensor of a gyroelectric medium, gyroelectric guided modes and their transverse optical spin are directly investigated. The effect of the thickness on the optical properties of the gyroelectric guided modes is investigated by varying the thickness of the slab within a range of 1 nm to 300 nm, which covers the thickness of monolayers of 2D-layered materials and conventional waveguides. We also demonstrate that a gyroelectric waveguide can be utilized as an optical spin selector/filter. These features are robust and unprecedented and offer a promising new strategy for the control of optical spin on-a-chip.
2. Transverse optical spin in a gyroelectric medium
In contrast to a conventional dielectric medium, a gyroelectric medium exhibits an anisotropic response to circularly polarized light. A gyroelectric medium has non-zero off-diagonal components in its dielectric tensor. One example of a gyroelectric medium is a ferromagnetic material with spin magnetization, and the sign of the off-diagonal components of its gyroelectric permittivity can be altered by the external magnetic field. This anisotropic permittivity induces important magneto-optic effects [17,18], such as the Kerr effect. There exist theoretical reports on optical guided modes in a gyroelectric waveguide [19–24] and optical spin quantization has been also theoretically proposed as a quantum gyroelectric effect [25]. However, the understanding of optical spin in a gyroelectric structure is still lacking despite of its importance.
In a gyroelectric medium, the monochromatic wave $\vec{E} = E{e^{i{k_x}x + i{k_y}y + i{k_z}z - i\omega t}}$ is governed by the Maxwell equation in a matrix form $KE = i\omega {\mu _0}H,\,\,KH ={-} i\omega \varepsilon E$, in which we assume $\mu = {\mu _0}$ for simplicity and the matrix $K$ and the gyroelectric permittivity tensor are
To manifest optical spin, we transform the Maxwell equation into a circular basis form:$\tilde{K}\tilde{E} = i\omega {\mu _0}\tilde{H},\,\,\tilde{K}\tilde{H} ={-} i\omega \tilde{\varepsilon }\tilde{E}$ where
The resulting wave equation has the simple form
The matrix $\tilde{A}$ is explicitly
This results in two solutions for ${k^2} = {q^2} + k_z^2$, which we call the slow and fast modes corresponding to the $+ $ and $- $ sign, respectively, in the following equation:
Remarkably, these modes possess transverse optical spin. We first recall that the standard expression of the optical spin density is given by $S = {\mathop{\rm Im}\nolimits} ({E^\ast } \times E)/2\omega $ [26] and the z-component ${S_z} = ({|{{E_ + }} |^2} - {|{{E_ - }} |^2})/2\omega $ (${E_ \pm } = {{({{E_x} \mp i{E_y}} )} / {\sqrt 2 }}$). To describe the transverse component of the optical spin explicitly, we set ${k_x} = 0$ in the wavevector $\vec{k}$ without loss of generality (Fig. 1(a)) and choose a specific transverse direction $\hat{n}$ normal to $\vec{k}$ by requiring that $\vec{k} \times \hat{n} \cdot \hat{z} = 0$ and the vector $\vec{k} \times \hat{n}$ points toward the positive x-direction. This choice of $\hat{n}$ is consistent with the conventional definition of tranasverse optical spin in a slab geometry. Then, the transverse spin component, normalized by intensity, is expressed by the degree of circular polarization (DOCP) about $\hat{n}$:
When we consider light propagation in a gyroelectric slab waveguide, unlike the bulk case, the nonvanishing component kz is required for the vertical confinement of light in the slab and the propagation direction is effectively given by the surface tangential component of the wavevector. Thus, to characterize transverse optical spin in a slab waveguide, we choose the z-axis as the transverse spin direction. To understand the transport behavior of transverse optical spin in a gyroelectric thin waveguide without a complicated analysis, we present here direct numerical analysis using a full 3D FDTD method, which we generalize to the case of a gyroelectric medium.
3. FDTD calculation for a gyrotropic waveguide
First, we extend the FDTD method [27] to include gyrotropic media. We introduce dispersive gyrotropy and/or transverse optical conductivity using the Lorentz-Drude model. The relevant Maxwell equations are
In later numerical calculations, we ignore conductivity and consider only the gyroelectric permittivity tensor $\hat{\varepsilon } = {\varepsilon _0}{\varepsilon _\infty } + \hat{\chi }$ given in Eq. (2). The corresponding finite difference equations for the n-th time step are given by following the conventional FDTD notation [23]
This modified FDTD equation is suitable for the real-time analysis of light propagation in a gyroelectric waveguide.
4. FDTD results
For numerical calculations, we consider light propagating through a planar slab waveguide made of a gyroelectric material, as illustrated in Fig. 2(a). We choose typical values for the Lorentz model parameters that are compatible with 2D materials(${{{\varepsilon _r}} / {{\varepsilon _0}}} = 23.4 + 3.6i$ and $\lambda = 650\,nm$), various values for ${\varepsilon _z}$ and $\alpha $, and a slab thickness of 1–300 nm. Because we consider a slab waveguide with symmetric refractive indices for the medium above and below the waveguide, there is no cut-off frequency for the fundamental guided mode. Near the outside edge of the slab, a soft line dipole source is applied to excite a symmetric mode inside the slab with maximum intensity at the center of the slab.
Figures 2(b)–(e) present the simulated salient features of the guided modes in a gyroelectric slab. The intensity profiles for different values of the gyro-factor $g = {\alpha / {{\varepsilon _r}}}$ and corresponding DOCP are presented in Figs. 2(b)–(d). Note that a vanishing gyro-factor ($g = 0$) exhibits a linearly polarized TE guided mode along a conventional dielectric waveguide. For $g \ne 0$, the effective refractive index of the guided modes depends on the gyro-factor, with the effective lateral wavelength increasing with a higher g. This occurs because the confining momentum ${k_z}$ of the slab is nearly fixed, which requires a smaller $q$ (i.e., a longer wavelength) for a higher g, as dictated by Eq. (9). We calculated the transverse optical spin density as the DOCP density about the z-axis as defined by
We also present the thickness-dependent behavior of guided modes in a gyroelectric slab, as shown in Fig. 3(a). As the thickness of the slab increases, more confined electric fields in the gyroelectric slab result in a higher optical spin density. When the spatial overlap between the electric field and the gyroelectric medium nears 100%, the optical spin density reaches its maximum and becomes saturated with increasing thickness. For a thicker slab, the calculated total optical spin density is robust, even though a thick gyroelectric waveguide supports not only fundamental but also higher modes. Explicit calculations indicate that the optical spin density is robust regardless of the number of guide modes. In addition, the transverse optical spin depends on the anisotropy (${\varepsilon _r} \ne {\varepsilon _z}$) of the slab, as depicted in Fig. 3(b). Because transverse optical spin appears as a consequence of the gyro-factor in the in-plane of the slab, a larger permittivity of the out-of-plane component (thus, ɛz) reduces the transverse spin density.
Finally, a gyrotropic mode carrying transverse optical spin plays an important role in manipulating optical spin on-a-chip. A gyroelectric waveguide couples to the left and right circularly polarized light with a different strength and subsequently acts as an optical spin sorter, as illustrated in Fig. 4(a). The explicit calculation of the transmittance of circularly polarized light in a gyrotropic slab is presented in Fig. 4(b). While the non-gyroelectric waveguide ($\alpha = 0$) has an identical response to each type of circularly polarized light, the gyroelectric waveguide has a preference for handedness depending on the sign of $\alpha$. The difference in transmission between two-handed circularly polarized light can reach up to ∼100%. This suggests that a gyroelectric waveguide can be an efficient optical spin selector/filter.
5. Conclusion
Until now, transverse optical spins were known to exist in localized EM fields and propagating plane waves can possess only longitudinal optical spins. In this work, for the first time we have theoretically proved that light in a gyroelectric medium can possess transverse optical spin. A gyroelectric waveguide can support the transport of transverse optical spin regardless of the propagation direction of light, which cannot be demonstrated with a conventional dielectric medium. A gyroelectric medium induces light to exhibit peculiar polarization properties. Longitudinal and transverse optical spin is sensitive to the direction of the light and the orientation of the gyroelectric medium. This unique nature of a gyroelectric medium can lead to the nonzero transverse optical spin of guided light even in a slab waveguide geometry, which is very different from linearly polarized TE or TM modes in a conventional waveguide. This transverse optical spin is also distinct from that of evanescence fields or chiral plasmon polaritons, which exist only at the edge of a system. The handedness of the transverse optical spin of gyroelectric guided modes is determined by the magnetization direction of the gyroelectric medium (thus the sign of $\alpha $) rather than the propagation direction of confined light. This robust and unprecedented polarization of gyrotropic modes offers the potential for a new approach to controlling optical spin on-a-chip and provides a new platform for the handedness-selective coupling of light with chiral molecules and spin/valley polarized emitters.
Funding
Samsung Science and Technology Foundation (SSTF-BA1902-03); National Research Foundation of Korea (NRF-2019R1A4A1028121).
Disclosures
The authors declare no conflicts of interest.
References
1. D. L. Andrews and M. Babiker, The angular momentum of light (Cambridge University Press, 2012).
2. L. Allen, S. M. Barnett, and M. J. Padgett, Optical angular momentum (CRC press, 2003).
3. L. D. Barron, Molecular light scattering and optical activity (Cambridge University Press, 2009).
4. Y. Tang and A. E. Cohen, “Optical chirality and its interaction with matter,” Phys. Rev. Lett. 104(16), 163901 (2010). [CrossRef]
5. S. Yoo and Q.-H. Park, “Chiral light-matter interaction in optical resonators,” Phys. Rev. Lett. 114(20), 203003 (2015). [CrossRef]
6. S. Yoo and Q.-H. Park, “Metamaterials and chiral sensing: A review of fundamentals and applications,” Nanophotonics 8(2), 249–261 (2019). [CrossRef]
7. M. Hentschel, M. Schäferling, X. Duan, H. Giessen, and N. Liu, “Chiral plasmonics,” Sci. Adv. 3(5), e1602735 (2017). [CrossRef]
8. M. Schäferling, “Chiral nanophotonics,” Springer Series in Optical Sciences 205, 159 (2017).
9. S. Barik, A. Karasahin, C. Flower, T. Cai, H. Miyake, W. DeGottardi, M. Hafezi, and E. Waks, “A topological quantum optics interface,” Science 359(6376), 666–668 (2018). [CrossRef]
10. T. Chervy, S. Azzini, E. Lorchat, S. Wang, Y. Gorodetski, J. A. Hutchison, S. Berciaud, T. W. Ebbesen, and C. Genet, “Room temperature chiral coupling of valley excitons with spin-momentum locked surface plasmons,” ACS Photonics 5(4), 1281–1287 (2018). [CrossRef]
11. T. Van Mechelen and Z. Jacob, “Universal spin-momentum locking of evanescent waves,” Optica 3(2), 118–126 (2016). [CrossRef]
12. K. Y. Bliokh, A. Y. Bekshaev, and F. Nori, “Extraordinary momentum and spin in evanescent waves,” Nat. Commun. 5(1), 3300 (2014). [CrossRef]
13. J. C. Song and M. S. Rudner, “Chiral plasmons without magnetic field,” Proc. Natl. Acad. Sci. 113(17), 4658–4663 (2016). [CrossRef]
14. L. Brey, T. Stauber, T. Slipchenko, and L. Martín-Moreno, “Plasmonic dirac cone in twisted bilayer graphene,” Phys. Rev. Lett. 125(25), 256804 (2020). [CrossRef]
15. S.-H. Gong, F. Alpeggiani, B. Sciacca, E. C. Garnett, and L. Kuipers, “Nanoscale chiral valley-photon interface through optical spin-orbit coupling,” Science 359(6374), 443–447 (2018). [CrossRef]
16. S.-H. Gong, I. Komen, F. Alpeggiani, and L. Kuipers, “Nanoscale optical addressing of valley pseudospins through transverse optical spin,” Nano Lett. 20(6), 4410–4415 (2020). [CrossRef]
17. Z. Qiu and S. D. Bader, “Surface magneto-optic kerr effect,” Rev. Sci. Instrum. 71(3), 1243–1255 (2000). [CrossRef]
18. T. Haider, “A review of magneto-optic effects and its application,” Int. J. Electromagn. Appl 7, 17–24 (2017). [CrossRef]
19. A. Eroglu and J. K. Lee, “Wave propagation and dispersion characteristics for a nonreciprocal electrically gyrotropic medium,” Prog. Electromagn. Res. 62, 237–260 (2006). [CrossRef]
20. S. Liu, L.-W. Li, M.-S. Leong, and T. Yeo, “Theory of gyroelectric waveguides,” Prog. Electromagn. Res. 29, 231–259 (2000). [CrossRef]
21. V. Mališauskas and D. Plonis, “Dispersion characteristics of the propagation waves in the gyroelectric semiconductor waveguides,” Elektronika ir elektrotechnika 106, 87–90 (2010).
22. E. Prati, “Propagation in gyroelectromagnetic guiding systems,” J. Electromagn. Waves Appl. 17(8), 1177–1196 (2003). [CrossRef]
23. L. Y. Tio, L. E. Davis, A. A. Gibson, and B. M. Dillon, “Novel general finite element solver for gyroelectric structures,” in IEEE MTT-S International Microwave Symposium Digest, 2003 (IEEE2003), pp. 421–424.
24. N. Uzunoglu, P. Cottis, and J. Fikioris, “Excitation of electromagnetic waves in a gyroelectric cylinder,” IEEE Trans. Antennas Propag. 33(1), 90–99 (1985). [CrossRef]
25. T. Van Mechelen and Z. Jacob, “Quantum gyroelectric effect: Photon spin-1 quantization in continuum topological bosonic phases,” Phys. Rev. A 98(2), 023842 (2018). [CrossRef]
26. K. Y. Bliokh, J. Dressel, and F. Nori, “Conservation of the spin and orbital angular momenta in electromagnetism,” New J. Phys. 16(9), 093037 (2014). [CrossRef]
27. A. Taflove and S. C. Hagness, Computational electrodynamics: The finite-difference time-domain method (Artech house, 2005).