Abstract
Employing a second-quantization of the electromagnetic field in the presence of media with both gain and loss, we investigate the propagation of the squeezed coherent state of light through a dispersive non-Hermitian multilayered structure, in particular at a discrete set of frequencies for which this structure is $\mathcal{PT}$-symmetric. We detail and generalize this study to cover various angles of incidence and s- and p-polarizations to reveal how dispersion, gain/loss-induced noises in such multilayered structures affect nonclassical properties of the incident light, such as squeezing and sub-Poissonian statistics. Varying the loss layers’ coefficient, we demonstrate a squeezed coherent state, when transmits through the structure whose gain and loss layers have unidentical bulk permittivities, retains its nonclassical features to some extent. Our results show by increasing the number of unit cells and incident angle, the quantum features of the transmitted state for both polarizations degrade.
© 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
Wave scattering by non-Hermitian structures has attracted a great deal of attention over the past two decades. Particular interest is devoted to the special class of non-Hermitian media, referred to as parity-time ($\mathcal{PT}$-) symmetric in quantum mechanics. $\mathcal{PT}$-symmetric systems are described by a Hamiltonian that is invariant under parity-time symmetry transformation. In a mathematical language, this means that if the Hamiltonian $\hat{H}$ commutes with the ${\mathcal{\hat{P}}{\hat{T}}}$ operator, $[{\hat{H},{\mathcal{\hat{P}}{\hat{T}}}} ]= 0$, and they share the same set of eigenstates, then the eigenstates $\hat{H}$ are entirely real [1–3]. For optical $\mathcal{PT}$-symmetric systems, the refractive index obeys the symmetry relation n(r)=n*(−r) wherein r and asterisk denote the position and complex operators [4–7]. This possesses the perfectly balanced spatial distribution of gain and loss for physical systems. The given symmetry is the only necessary condition for the so-called “exact” phase or $\mathcal{PT}$-symmetric regime. The $\mathcal{PT}$-symmetry exact phase regime sustains when the gain/loss strength remains below a threshold, known as the exceptional point. Otherwise, the $\mathcal{PT}$-symmetry broken phase regime prevails, resulting in a complex eigenvalue spectrum [1–7].
Extension of $\mathcal{PT}$-symmetry to systems with eigenvalues that correspond to the scattering matrix has led to some novel phenomena: optical switching [8], nonreciprocal propagation [9,10], unidirectional reflectionless transmission [11,12], unidirectional invisibility [13–15], some extraordinary nonlinear effects [16–18], extraordinary transmission and reflection [19], optoelectronic oscillators [20], and phase transition in $\mathcal{PT}$-symmetric active plasmonic systems [21]. All these make use of classical electromagnetic waves. Despite the successful implementation of $\mathcal{PT}$-symmetry in the classical systems, some controversial results are proposed in the full-quantum regime, such as ultrafast states transformation and violation of the no-signaling principle [22,23]. However, investigations on the interaction of quantum waves and matters have left open the question of “whether the light retains its quantum features, after the interaction.”
Nonclassical states of light, such as squeezed states, can provide distinct properties, like reduced noise and strong correlations [24] compared with classical light and have found numerous applications in sensing and quantum metrology beyond the fundamental limits of precision set for classical light [25,26]. The quantum states of light propagating through absorbing or amplifying media are affected by quantum noise associated with the loss and gain [27–35]. Unlike in classical optics, so far, a few reports have explored the potential benefits of $\mathcal{PT}$-symmetric bilayers in quantum optics [35–40]. In our most recent work [35], we extensively studied the quantum states of light normally propagating through a dispersive non-Hermitian bilayer structure. There, we have demonstrated how the dispersion and the gain(loss)-induced noises in such structures affect the incident light quantum features, like squeezing and sub-Poissonian statistics. Then, we have demonstrated below a critical value of gain quantum optical effective medium theory (QOEMT) correctly predicts the behavior of quantized waves propagating through the non-Hermitian bilayer. We have also shown that unidirectional invisibility cannot be realized in quantum optics.
In nonclassical optics, the general case of non-normal incidence is of interest since the scattering patterns strongly depend on the angle of incidence. In addition, we know the propagating behavior of the s- and p-polarized waves differ qualitatively for oblique incidences [28]. Motivated by the results of [35], obtained from a one-dimensional analysis of a non-Hermitian bilayer under normal incidence, we aim at a more general investigation providing deeper insight into the physics of non-Hermitian periodic structures beyond the first quantization. In doing so, by investigating the properties of s(p)-polarized squeezed state of light obliquely propagating across a non-Hermitian multilayered structure, here, we evaluate the nonclassical features like quadrature squeezing and the photon counting statistics of the transmitted light for various loss coefficients and incident angles. We study the effects of the dispersion and the loss(gain)-induced noises on the squeezing and sub-Poissonian statistics for s(p)-polarization in the exact-phase and broken-phase regimes. This examination can serve as a meaningful tool to more accurately assess the realization of $\mathcal{PT}$-symmetry in quantum optics. Our results can have many applications, specifically, those based on manipulating the photonic spin Hall effect with nonclassical light [41], wave propagation, and polarization control, like polarization rotators [42] and polarization modulators [43].
2. Method
2.1 Multilayered structure
Consider a finite non-Hermitian multilayered (Fig. 1) composed of a few pairs of homogeneous gain/loss nanolayer of the same thickness (l) infinitely extended in the x-y plane. The structures with the total thickness of L = (N−1)l is surrounded by the vacuum along the z-direction at | z | > L/2. The background dielectric permittivity of gain (loss) medium, εg(l), follows the Lorentzian form [44],
The plasmonic metamaterial with a lossless glass substrate wherein the quantum noise flux vanishes can provide an experimental proposal for this structure [46–48].
2.2 Exact multilayer theory
Assume an s(p)-polarized quantum state of light impinging at an angle of incidence, θ, from the left (right) upon the multilayered structure. According to the second quantization formalism of the electromagnetic field, the transverse positive Fourier component of the electric field operator in the jth layer is [28]:
The explicit forms of ${\hat{F}_{R(L),\sigma }}$ and the scattering matrix elements can be found in [28]. Similar commutation relations for the output amplitude operators can be derived by substituting (3) in (4).
3. Results and discussion
In our investigations, we have considered two sets of unit-cells, with physical parameters given in Table 1 to constitute the multilayered structure of Fig. 1. These parameters are the same as those used in [44,49]. As listed in this table, the gain and loss layers with the same thickness (l = 10 nm) for Set 1 (Set 2) have identical (unidentical) background permittivities. In other words, Δε = εbl − εbg = 0 (1.22) for Set 1 (Set 2).
According to Eq. (1) and Table 1, the frequency, the loss, and the gain parameters that satisfy the $\mathcal{PT}$-symmetric necessary condition for Set 1(Set 2) are $\omega = \omega_{\mathcal{PT}} = \omega_{\rm 0g}$ (1.58 ω0g) for any arbitrary value of αl =| αg | (solely for αl = 2 and αg = −20.86). We use the given parameters to investigate the behavior of the outgoing optical beam at z = zN (z1) when an s(p)-polarized quantum state obliquely impinges from the left (right) upon the slab z = z1 (zN).
3.1 Scattering matrix eigenvalues
In general, for both polarizations, the eigenvalues of the scattering matrix (3) for the exact $\mathcal{PT}$-symmetric phase are unimodular, fulfilling the condition |λ1,σ λ2,σ| = 1. Hence, up to the so-called exceptional-point we have |λ1,σ| = |λ2,σ| = 1, beyond which the broken phase regime emerges, and the eigenvalues become an inverse conjugate pair, satisfying the relation $|\lambda_1, \sigma|$=| λ2,σ |-1 > 1 (i.e., the so-called $\mathcal{PT}$-broken phase) [5,11]. From Eq. (3), we can write the eigenvalues for a unit-cell (a bilayer):
To identify whether the system lies in the $\mathcal{PT}$-symmetric or $\mathcal{PT}$-broken phase, we examine the dependency of the eigenvalues difference, Δλσ = | λ2,σ | − | λ1,σ |, on the loss coefficient (αl) and the incident angle (θ) for both polarizations. We assumed an s(p)-polarized quantum state impinging upon the structure of Fig. 1 composed of Set 1 unit-cell at an arbitrary angle θ and calculated the corresponding eigenvalues versus θ and αl. Figures 2(a) and 2(b) illustrated Δλσ in the (θ, αl) plane for s- and p-polarization. As shown in this figure, for any given value of 0 ≤ θ ≤ 85° and αl < 890, the $\mathcal{PT}$-symmetric exact phase regime for both polarizations prevail (i.e., Δλσ = 0). Moreover, the exceptional point occurs at αl = 890 (marked with vertical dashes), beyond which the so-called broken phase occurs for both polarizations at any given angle of incidence. This case is contrary to that reported for the chiral $\mathcal{PT}$-symmetric materials [50–52], in which s- and p-polarizations showed different exceptional points at any given incident angle except θ = 0°. Figure 2(c) and 2(d), illustrating λ1,2(σ) versus αl for θ = 30° and 60° manifest the nature of the eigenvalues in each regime. Being unimodular in the exact phase regime and nonunimodular in the broken phase regime. Further comparison shows, unlike the exact-phase eigenvalues, those of the broken-phase depend on the incident angle and polarization.
As we have pointed out earlier in this section, the Set 2 unit-cell only at αl = 2 (| αg | = 20.86), the condition | λ1,σ | = | λ2,σ | = 1 is satisfied. Otherwise, this unit-cell cannot be $\mathcal{PT}$-symmetric for any given angle of incidence and polarization (see [35]). In the following subsections, we investigate how quantum features of the incident state (here, the squeezing and sub-Poissonian statistics) are degraded in the $\mathcal{PT}$-symmetry and also in the broken phase regimes for Set 1 and Set 2.
3.2 Quadrature squeezing
In this section, we study how propagation through the multilayered structure influences the squeezing of the incident light. In doing so, we take the state of the quantized field |L〉=|0〉 (a conventional vacuum) impinging leftward and |R〉 (a squeezed coherent continuous-mode) impinging rightward upon the multilayered structure. The balanced homodyne detector (shown on the right-hand side of Fig. 1) can measure the quadrature squeezing of the scattered light. In other words, a 50-50 beam splitter mixes the outgoing light from the structure with the coherent mode of the local oscillator (LO) of frequency ωLO and phase ϕLO. Consider a narrow-bandwidth homodyne detector is functioning during a sufficiently long-time interval [27–31]. After some lengthy mathematical manipulations, one can obtain a compact formula for the variance of the difference between the photocurrents given by [28,31],
Next, we have repeated similar calculations for non-Hermitian structures, made of (a) one and (b) four unit-cells designated by Set 2 (see Fig. 4). As seen from this figure, there are specific regions in the αl−θ plane over which the transmitted states through these non-Hermitian structures for both polarizations remained squeezed. A careful comparison of the data in Figs. 4(a) and 4(b) reveal that as the number of the constituting unit-cells in these multilayered structures increases, the area of the corresponding squeezed region decreases. This phenomenon is due to the significant increase in the quantum noises within the structure originating from the gain layers at 0 K. Unlike for Set 1, the quantum noise for Set 2 at the incident frequency of ωLO =1.58 ω0g is negligible, having little effect on the squeezing property of the incident state. In other words, the transmitted states through these multilayered structures, to some extent, retain the squeezing property of the incident states.
The regions in Fig. 4(a) and 4(b) enclosed by the green dots represent the squeezed region. Notice, these non-Hermitian structures behave like lossless (gainless) structures with negligible reflectances (RR ≈ RL < 30%) and large transmittances (T > 80%) for small values of αl and the given range of θ (see Fig. S2 in Supplement 1). This property makes the noise flux vanishingly small, which adds up with the small positive values of the transmission-related term (i.e., the third term on the right-hand side in Eq. (6)), contributing to the squeezing variance to make it slightly greater than one. A moderate increase in αl, results in a dominantly negative transmitted-related term due to the presence of the αl-dependent phase, ϕt, resulting in 〈(Δ$\hat{E}$)2〉σout < 1. As αl exceeds a particular value, at any given θ, each of these two non-Hermitian structures behaves like a partial mirror with RR ≈ RL > 80% and T < 20% for both polarizations (see Fig. S2, in Supplement 1). This behavior forces the scattering mode to approach the vacuum state with the variance of 〈(Δ$\hat{E}$)2〉σout ≈ 1, at large αl values.
Comparing the six plots in Figs. 3(c) or 4(c), we realize that the magenta and blue dashes (representing θ = 0 for s- and p- polarizations) in either figure coincide over the entire range of the given αl. In other words, the light polarization does not affect the propagation of the normally incident quantum states passing through either of the two sets of non-Hermitian multilayered structures (Set 1 and Set 2), as expected. Nonetheless, the deviation of magenta dotted and solid lines from their blue counterparts in each figure indicate that the former statement is not valid for oblique incidences (i.e., θ > 0). Moreover, we can see as the θ increases, the variance spectrum for the s(p)-polarization compresses (expands) towards smaller (larger) αl, with a larger (smaller) minimum.
It is worth noting that the incident and transmitted light through the non-Hermitian structure (constituting loss/gain unit-cells) designated as Set 1 are not equivalent. Despite the apparent simplicity of our example, it does have far-reaching consequences for any attempt to study $\mathcal{PT}$-symmetry of quantum optical systems. First of all, the gain layer, regardless of its spatial distribution, always adds thermal noise to a quantum state at zero temperature. Second, we have chosen squeezed states that are minimum uncertainty states while having the unique property, such that loss cannot affect their purity. For example, pure photon-number states turn into mixed states with lower photon numbers. Hence, any quantum state of light is crucially altered when propagating through Set 1 structures. In other words, Hamiltonians for such non-Hermitian structures do not commute with the $\mathcal{PT}$ operator (i.e., $[{\hat{H},\hat{P}\hat{T}} ]\ne 0$); and the nonclassical features of transmitted light are entirely lost. Nonetheless, the quantum states of light after transmitting through the non-Hermitian structure of Set 2 can preserve their nonclassical features to some extent for some given values of αl and θ. This is an apparent manifestation of broken $\mathcal{PT}$ -symmetry in quantum optics as far as the squeezing feature of the outgoing light is concerned.
3.3 Photon counting statistics
The so-called Mandel parameter is a practical tool for characterizing the photon counting statistics in the transmitted nonclassical light field through the multilayered structure [31]. Using a photo count detector with a Gaussian filter of bandwidth σH and center frequency ωH, in which ωH ≫ σH, one can measure the photon counting statistics. Moreover, after some lengthy manipulations, the Mandel parameter becomes
Figures 5(a) and 5(b) illustrate the profiles of the Mandel parameter (Qσ / Q0) in the αl-θ plane obtained at 0 K for the Set 1 made of (a) one and (b) four unit-cells for the (i) s-polarized and (ii) p-polarized output states. As shown in Fig. 5(a) and 5(b), a vast area in the αl-θ plane corresponds to the super-Poissonian statistics for s- and p-polarizations. That is because of the significant quantum noises within this set of the $\mathcal{PT}$-symmetric structures at ω = ω0g and the given range of αl−θ. Moreover, the Mandel parameter distribution for each case (i or ii) may vary from one polarization to another. One can attribute this variation to the differences in the corresponding transmittances and the right (left) reflectance for the obliquely incident s-and p-polarized lights (see Fig. S1 in Supplement 1). For example, in a particular area of the αl−θ plane, the profile in Fig. 5(a-i or b-i) may represent sub-Poissonian statistics. While, in a similar region, Fig. 5(a-ii or b-ii) may represent super-Poissonian statistics and vice versa. This dependency demonstrates the possibility of controlling the quantum features of the transmitted light through non-Hermitian systems by polarization. The green dots in Fig. 5(a) and 5(b) represent the boundaries between sub-Poissonian and super-Poissonian regions —i.e., the loci of Qσ = 0. A further inspection shows, an increase in the number of unit-cells constituting the structure expands the area covered by super-Poissonian distribution for both s- and p-polarized states. This phenomenon is due to the significant quantum noises within the Set 1 structures originating from the gain layers at 0 K.
Again, we focus on three particular angles — i.e., at θ = 0°, 30°, and 60° — and extract data from Figs. 5(b) to further compare the dependency of Qσ / Q0 on the loss coefficient, αl, at the given angles of incidence for the structures made of four unit-cells of Set 1, as depicted in Fig. 5(c). The inset in this figure shows only for small values of αl the photon statistics are sub-Poissonian (Qσ / Q0 <0), while the squeezing character is not retained (see Fig. 3 (c)). Here too, alike in Fig. 3(c), the magenta and blue dashes coincide over the entire range of the given αl, meaning the propagation of normally incident (θ = 0°) quantum states through a planar structure are polarization independent. Recall that for large values of αl, this set of structures multilayers perform as a mirror for both polarizations. Albeit, the Mandel parameter for any given angle of incidence is slightly greater than zero at αl = 1000.
Now, we move to Set 2, investigating the variations of the Mandel parameter, similar to those shown in Fig. 5 for Set 1. Figure 6 shows these variations versus αl and θ for the s- and p- polarized states transmitted through Set 2 non-Hermitian structures made of (a) one and (b) four unit-cells at ωLO = 1.58ω0g. As can be seen from this figure, this set of non-Hermitian slabs, unlike Set 1, preserves the sub-Poissonian statistics of the incident states for both polarizations, over the entire given αl-θ plane. The dots in Fig. 6(a) and 6(b) represent the boundaries between sub-Poissonian and Super-Poissonian statistics — i.e., the loci of Qσ=0. This effect can be seen more clearly from plots of Fig. 6(c), depicting the dependence of the Mandel parameters on the loss coefficient, at θ = 0°, 30°, and 60°. One can attribute this phenomenon to the incident frequency being far away from the emission frequency of the gain layers in the Set 2 structure, making the quantum noise infinitesimal, even at αl = 1000. Moreover, the difference between profiles of the Mandel parameters for different polarizations corresponds to the difference in their related transmittances and right and left reflectances in the similar range of αl,observed in Fig. S2 for one unit cell. Recall the Set 2 structure behaves like a lossless (gainless) structure with negligible reflectances and large transmittances for small loss values. Nonetheless, it acts as a mirror at the large values of αl. The latter behavior forces the scattering mode to approach the coherent state with a zero Mandel parameter for large loss values. The results of Fig. 6(c), as far as the dependence of the Mandel parameter on the incident polarization and angle is solely concerned, show that the structure composed of Set 2 is a suitable candidate to realize the $\mathcal{PT}$-symmetry in quantum optics.
4. Conclusions
We have investigated the behavior of obliquely incident s- and p-polarized quantum states after transmitting through dispersive non-Hermitian media. To account for the dispersive, dissipative, and amplification properties, we employed the Lorentz model. Then, considering a squeezed coherent state of light with an arbitrary angle of incidence, we have investigated to see to what extent the transmitted light could retain its original nonclassical features, like the quadrature squeezing and sub-Poissonian photon statistics. In doing so, we have considered two sets of non-Hermitian structures: one with gain/loss layers of identical background materials (Set 1) and the other with unidentical background materials (Set 2). The frequencies of the incident squeezed coherent states were equal to the frequencies satisfying the $\mathcal{PT}$-symmetric necessary condition for both sets, which equals the emission frequency of gain layers in Set 1 (ωLO = ω0g) and is far away from Set 2 (ωLO = 1.58ω0g). Our findings for one unit-cell show that Set 2 can retain the sub-Poissonian photon statistics (squeezing) of the incident squeezed coherent states, to some extent over the entire (some parts of) αl-θ plane for both s- and p-polarizations. However, Set 1 cannot retain the squeezing (sub-Poissonian photon statistics) of the incident squeezed coherent states over the entire (large parts of) αl-θ plane. Hence, one cannot implement $\mathcal{PT}$-symmetry, at any arbitrary angle of incidence for either polarization in the quantum optics domain as far as the squeezing feature of outgoing light is concerned. Although, this situation is changed if one only probes the sub-Poissonian photon statistics of outgoing light, and it seems that the structure composed of Set 2 is a good choice. We have also found that for both polarizations, the quantum features of the transmitted state degrade as the number of unit-cells constituting the structures and the incident angle θ are increased. Moreover, the transmitted quantum states of light through these non-Hermitian multilayers have not behaved extraordinarily at exceptional points.
Funding
Tarbiat Modares University (IG-39703).
Acknowledgments
This work was supported by Tarbiat Modares University (TMU) (IG-39703).
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper may be obtained from the authors upon reasonable request.
Supplemental document
See Supplement 1 for supporting content.
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