Abstract
A proposal is made for the generation of polarization-entangled photon pairs from a periodically poled crystal allowing for high collection efficiency, high entanglement, and stable operation. The theory is formulated for colinear propagation for application to waveguides. The key feature of the theory is the use of type II phase matching using both the +1 and −1 diffraction orders of the poling structure. Although these conditions are fairly restrictive in terms of operating parameters, practical operating conditions can be found. For example, we find that a HeNe pump laser may be used for a periodically poled rubidium-doped potassium titanyl phosphate (Rb:KTP) waveguide to yield single mode polarization-entangled pairs. Fidelities of 0.98 are possible under practical conditions.
©2011 Optical Society of America
1. Introduction
Photonic entanglement is essential to the study of fundamental physics and quantum information science. Polarization is frequently used as the entanglement degree of freedom although other variables such as momentum, orbit-angular-momentum, time and energy are also choices. Many pioneering experiments such as a non-locality test [1] and quantum teleportation [2] were explored using polarization-entangled photons. Recently field tests for quantum-key-distribution with polarization-entangled photon pairs have begun [3]. These applications demand the development of a simple, high quality source of polarization-entangled photon pairs. We propose and model a new scheme that offers efficient collection, high entanglement fidelity, and stable, convenient operation.
While the principle has been around for a long time [4], the most common sources of polarization-entangled photons still create pairs via spontaneous parametric down conversion (SPDC) in nonlinear crystals, and advances continue to be made. The basic design has been to effectively create two pair sources with orthogonal polarization and place them so that one cannot determine which source generated the pair other than through the emitted polarization thus yielding entangled pairs. The first such source used type-II phase-matched SPDC in which the down-converted photons were emitted into two non-concentric cones, one with ordinary polarization and the other with extraordinary polarization. These two cones intersect along two lines with polarization-entangled photon pairs collected only along those two special angular directions [5]. In 1999, Kwiat and his colleagues demonstrated a new source scheme using type-I SPDC where an extraordinary polarized pump produces two photons that have matching ordinary polarizations [6]. They stacked together two such identical thin nonlinear crystals but rotated one crystal 90° about the pump direction. The pump laser beam is linearly polarized at 45° with respect to both crystals’ extraordinary axes. Half of the pump beam light drives a type-I parametric down-conversion process in one crystal; the other half drives an identical type-I parametric down-conversion process in the second crystal, but with polarizations of pump and two daughter fields orthogonal to the corresponding fields in the first crystal. The entire emission cones of the two type-I parametric processes nearly perfectly overlap each other. Polarization-entangled photon pairs can be selected from any azimuthal angle around the axis of the cone. This bright source allows many interesting applications such as high-dimensional entanglement [7] and hyper-entanglement [8]. A new polarization-entangled-pair source development was contributed recently by Kim, Fiorentino, and Wong [9]. They placed a periodically poled Potassium Titanyl Phosphate (PPKTP) crystal in a Sagnac interferometer. Pump beams entering each end of the crystal coherently drove two identical type-II SPDC processes. The Sagnac arrangement combines the output of the two SPDC processes so that the creation direction cannot be determined, the yielding entangled photon pairs. The advantage of this source is that all beams propagate coaxially, greatly easing the optical alignment including the collection of entangled photons which has been cumbersome in previous sources.
In this paper, we propose a new source scheme for polarization-entangled photon pairs, one which builds on the two-source theme of Kwiat and co-workers [5, 6] and Kim et al. [9] by effectively creating two sources within a single crystal and using only a single pass of the pump laser beam through that crystal. With a proper choice of poling period and a simple compensation of the temporal walk-off, an entanglement fidelity near unity can be achieved.
Our scheme, shown in Fig. 1, employs a periodically poled waveguide in which two different type-II SPDC processes occur. Each of the processes are quasi-phase matched type II SPDC but the poling contributes a wave vector of opposite sign for the two different processes, as illustrated in Fig. 1(b). Typical optics for a two-photon coincidence experiment are shown in Fig. 1(c). This arrangement takes advantage of the high two-photon brightness made possible by quasi-phase matching and periodic poling and a waveguide geometry is used to limit the pair production to a single spatial mode. The waveguide is formed by the diffusion of Rb [10] into KTP which displaces some of the K ions in the lattice, forming and an alloy of Rubidium Titanyl Phosphate (RTP) and KTP varying from pure RTP at the surface to pure KTP at a depth of tens of micrometers. (We denote this system as an Rb:KTP waveguide.) The complexity of the alignment is much reduced compared to previous sources, leading to superior stability and high fidelity.
2. Polarization-entangled two-photon state in a crystalline waveguide
Quasi-phase matching has been extensively applied in SPDC to create photon pairs at chosen wavelengths [11]. In quasi-phase matching, the domain of the crystal of length L = 2ℓ is reversed in a pattern with period Λ, called the poling period, so that the usual wave vectors of phase matching are supplemented by wave vectors corresponding to 2π/Λ times an integer m [12]. If the pattern is chosen to correspond to a square wave with a 50 % duty cycle, then the additional spatial frequencies are 2mπ/Λ but include only the integer pairs m = ±1, ±3. To avoid an edge effect, L should be in an integral multiple of Λ, although L >> Λ is a sufficient condition. (Hereafter we will not distinguish between phase matching and quasi-phase matching.)
Spontaneous parametric down conversion in a waveguide which supports only a single mode for the daughter photons yields a two-photon state which may be written as
where the spatial integral is taken over the waveguide, the angular frequencies are each integrated from −∞ to ∞, β(ωs, ωi) is a two-photon joint spectral amplitude, where ωs and ωi are the frequencies of the signal and idler fields, Uj(r⃗,ω) is the spatial mode of the waveguide, for polarizations along crystal axes is the creation operator for a photon at a point r⃗ with angular frequency ω and polarization j, and |0〉 is the photonic ground state. We use the convention that a bar over a state is unnormalized. We consider the case in which the confined modes at both the signal and idler frequencies are unique (i.e., single mode) for each of the two polarizations. The effect of the slightly different spatial modes for each polarization proves to be modest, so we defer its treatment to Appendix A. Neglecting the effect of spatial modes, Eq. (1) reduces to where the creation operators create photons in a mode with a fixed spatial dependence.The pump photon with angular frequency ωp turns into a signal and idler photon pair. Energy is conserved, so ωp = ωs + ωi. If we consider parametric down conversion in a straight crystalline waveguide or a bulk crystal of length L = 2ℓ, the joint spectral amplitude is given by
Here, α(ωp) is the pump spectrum, sinc[Δkm(ωs, ωi)ℓ] is a phase matching function, and the cm are taken to be constants [13].A typical choice for the pump spectrum in Eq. (3) is the Gaussian
where is the central pump angular frequency and σp is the width. We have chosen the constants in Eq. (4) so that for the CW case We only consider the CW case in this paper.A key feature here is that we assume c 1 ≈ c– 1 in Eq. (3) and that all the other cm may be neglected. (The first assumption is justified in Appendix B. The terms cm with |m| > 1 may be neglected because the effective nonlinear coefficient d eff = 2d bulk /(|m|π), so the m = ±1 terms are the largest; moreover, the other terms lead to phase matched frequencies which are different from those of m = ±1 and are removed by spectral filtering of the light, as shown in Fig. 1(c).) Our goal is to find conditions so that both the m = 1 and m = −1 terms support parametric down conversion simultaneously, with these two processes being the heart of our entangled photons source. The case using type-0 SPDC with m = 0 and type-II SPDC with |m| = 1 has been implemented experimentally [14].
The wave vector mismatch in Eq. (3) is given by
for type II phase matching in a periodically poled crystal with poling period Λ; the choice of Λ is set by our use of periodically-poled KTP with Y and Z representing directions of polarization in the crystal. The wave vectors are defined by kj(ω) = ωnj(ω)/c, where nj(ω) is the index of refraction for the polarization indexed by j, and c is the speed of light.The two-photon joint spectral amplitudes β(ωs, ωi) will be largest when ωp is centered on angular frequency for which . In order to achieve a polarization-entangled state, we select an operating point such that
i.e., and , which implies . The situation is illustrated in Fig. 2 for a case studied in the next section.We develop a Taylor series about these points, introducing detuning frequencies , , and . Expanding about these points
hence where the function and the primes denote differentiation with respect to the argument. In the special case , where we have swapped the order of the arguments ξs and ξi as well as eliminating the variables in favor of .Introducing the times
we may write These times are the difference of the transit times for the pump and another mode across half of the crystal. This completes the formalism related to linearizing Eq. (3).Fidelity of entanglement
We develop an analytic formula for the fidelity of an entangled state and follow up in the next section with numerical results for a particular Rb:KTP waveguide.
Interchanging the variables of integration ωs ↔ ωi in Eq. (2) and then interchanging the order of integration, we may write
If we define two additional unnormalized two-photon states we find these states are related by using Σ± 1 = 2 and Σ± ±1 = 0.The normalized state from Eq. (2) is written
and, similarly, for Eq. (14), . For an ideal polarization-entangled state, corresponding to β(ωs, ωi) = ±β(ωi, ωs). By considering the relevant matrix element of creation and destruction operators, the orthogonality relation may be derived and soThe fidelity of a state is defined as F = Tr{ρ|2〉〈2|} [15]. We will focus on to the case of the symmetric state by using the density matrix ρ = |2+〉〈2+|. (Any other choice of ρ leads to a lower figure for the fidelity assuming we are testing for the dominant state.) Substituting this form for ρ into the fidelity formula leads to
using Eq. (16), Eq. (17), and . The problem of finding the fidelity F has reduced to the evaluation of because of Eq. (17).We need the matrix element
to write As discussed in Appendix A, the foregoing discussion needs to be modified for a waveguide to take into account the differences in the spatial modes. Next, we define the direct integral and the exchange integral In terms of the direct and exchange integrals, The fidelity is given by using Eq. (17), Eq. (18), and Eq. (26).The integrals I and J are evaluated in Appendix C, leading to the expression
using the symbols defined near Eq. (42). Eq. (25) implies . The maximum value F = 1 is achieved when Δτ + = Δτ–. Restated, we obtain a high fidelity symmetric state when |τ 1 s – τ 1 i| ≈ |τ− 1 s − τ− 1 i|, or equivalently, when . In the limit of zero pump bandwidth (i.e., a CW source), F is independent of both and the crystal length L = 2ℓ. While the natural range of F is 0 to 1, the assumption c 1 = c– 1 limits the range of F. Although we do not explore it here, c 1 = − c− 1, leads to and is relevant for generating a pure state |2−〉.3. Fidelity of polarization-entangled states for our source
We propose and explore an operating point for our periodically-poled KTP (PPKTP) waveguide. We chose this medium for our waveguide because it has been used previously for SPDC-based sources in waveguides [14,16,17] and in the bulk [18,19]. In our proposed system, shown in Fig. 1, a pump laser (possibly HeNe) is coupled to a waveguide formed from Rb diffused into a periodically-poled KTP crystal. Polarization-entangled signal and idler waves are generated through parametric down conversion. Upon exiting the crystal, the pump wavelength is removed from the beam. These waves pass through a bulk KTP crystal rotated by 90° for pulse timing compensation [5, 16, 20].
The index of refraction is usually parametrized using a Sellmeier equation. For KTP, we follow König and Wong [24] who recommend the Sellmeier equation of Fradkin et al. for [25] and who introduce a new Sellmeier equation for . For the difference in the indices of KTP and RTP, for j = Y,Z, we use the measurements of Cheng et al. [26] who reports values for both crystals with one set of instruments. The index of refraction for the bulk crystals is given in Fig. 3. We followed this mixed procedure because the Sellmeier equation of König and Wong was developed specifically for PPKTP. This Sellmeier equation accounts for the reported type-0 phase matching for SHG in PPKTP as shown in Table 1.
We calculated the effective index of refraction for waveguides with Rb diffused into KTP (Rb:KTP) using the Sellmeier equations given above and the commercial software package Comsol Multiphysics including its RF (Radio Frequency) Module [27]. The waveguide parameters are the width w and the profile of the Rb dopants whose index profile decreases with depth into the crystal from the bulk RTP value to the bulk KTP value following the function erfc(−Z/Z 0) [28] where the crystal surface is at Z = 0, and Z = 0 in the waveguide and in the crystal. We used a simulation region consisting of two quarter-circles filled with KTP with a 20 μm radius, a rectangular region of width w between the quarter circles to represent the waveguide proper, and a rectangular region of (40 μm +w) × 4 μm above to represent the air. A sketch of the simulation region is shown in Fig. 4 (top), along with the variation of the index of refraction in a particular case (bottom left). On the boundary, the fields were required to vanish. This approximation causes little error because the fields were exponentially confined. The simulation region was large enough that boundary effects were negligible as tested by comparing to a 30 μm radius boundary in selected cases and by visual inspection of the confined modes. The parameter w was chosen to ensure that the down converted photons are in a single mode for the signal and the idler.
In the standard approach, a crystal used for dispersion compensation matches the source crystal except for being half their length and rotated by 90° [5]. Here, to avoid the necessity of coupling into a second PPKTP waveguide, we propose using a rotated bulk KTP crystal instead. The compensation is adequate even though the materials are not exactly matched. For the case of a waveguide shown in Fig. 1, with a poling period Λ =1 mm, λs = 1247 nm and λi = 1284 nm. The spread in the wave packet arises because photons converted near the exit face of the waveguide exit at almost the same time, whereas those converted near the entrance of the waveguide exit with a time difference given by (L/c)[nZ(λs) − nY (λs)] or (L/c)[nZ(λi) − nY (λi)], corresponding to 0.08069L/c and 0.08083L/c. For the bulk crystal, the corresponding figures are 0.08325L/c and 0.08348L/c. With a single length for the bulk crystal, we may compensate the average delay by choosing the bulk crystal length to be 0.9688/2 of the waveguide instead of the traditional 1/2. This deviates from the ideal compensation by ±2 × 10−5 L/c, which is only 2.5 × 10−4 L/c of the broadening by the waveguide. Hence, we conclude that bulk KTP may be used to compensate the timing of the broadening of two-photon wave packets in the KTP waveguides in analogy with the standard compensation scheme. For reference, if L = 10 mm, then L/c = 33 ps, the delay is about 2.6 ps, and the compensation error is about 0.7 fs.
We estimate that the conversion of photons from higher pump modes is negligible. Some of the higher pump modes will have odd parity under crystal Y ↔ –Y about the waveguide centerline and hence yield a vanishing triple mode integral, yielding no signal and idler photons. The first higher mode with even parity, the third mode overall, yields a triple mode integral of 39 % that of the fundamental mode integral at (λp, λs, λi) = (625, 1250, 1250) nm, and this factor enters the production rate squared, i.e., 0.15. Coupling to the input pump beam is likely to be weak compared to coupling to the fundamental pump mode of the waveguide. Finally, the effective index of refraction of this higher pump mode is 1.871 vs. 1.786 for the fundamental mode at λp = 625 nm, suggesting the higher mode’s signal and idler photons will be generated far from phase-matching conditions.
When the wave vector mismatch given in Eq. (6) vanishes, the phase matching condition is satisfied. The poling period Λ required to achieve phase-matched degenerate SPDC in bulk KTP and a periodically poled waveguide of width w = 3.5 μm and Z 0 = 4.5 μm with the parameters defined in Table 2 is shown in Fig. 5. The poling periods required for type II phase matching are much longer than that needed for type 0 phase matching. This may be understood because the higher index of refraction for the Z polarized wave partially cancels the higher index of the (short wavelength) pump. Varying w or Z 0 has a very modest effect on the results as shown in Table 2. This Table also shows it is possible to obtain phase-matched degenerate SPDC with a HeNe laser λp = 632.8 nm for certain values of (w,Z 0) such as (3.4,4.5) μm and (3.7,4.5) μm.
The signal, idler, and (doubled) pump wavelengths are shown in Fig. 6 as a function of the poling period Λ. To obtain Fig. 6 it was necessary to find the intersection points of curves Δk(ωs, ωi) = –Δk(ωi, ωs), illustrated in Fig. 2 for the case of Λ = 1 mm. Because we are imposing the constraints of Eq. (7), once the material, geometry, and Λ are chosen, there are no additional degrees of freedom. Hence, it is fortunate that the wavelengths are reasonably convenient, and that, with carefully chosen parameters, operation with HeNe laser for the pump should be possible. The curves are given for room temperature. The curves for the KTP are shifted upwards by about 0.6 nm for a 20 C rise above room temperature. Curves for RTP and the waveguide are similarly affected. The temperature coefficients for the index of refraction were taken from Emanueli and Arie [29] for KTP and Mikami et al. for RTP [30].
Next, we come to the main goal of this paper, the estimate of the fidelity of the polarization-entangled states, according to Eq. (25). The results for KTP, RTP, and an Rb:KTP waveguide are shown in Fig. 7. (We have assumed colinear propagation, so the meaning of the results for the bulk crystals is hypothetical.) The main point is that high fidelities may be achieved for long poling periods. For example, for Λ = 1 mm, a fidelity of 0.987 may be achieved in the wave-guide for (λp, λs, λi) = (632.6, 1246.8, 1284.1) nm. As the poling period becomes increasingly long, the signal and idler wavelengths become more similar, as shown in Fig. 6.
The condition in Eq. (36) becomes increasingly important as Λ → ∞, the small parameters growing from about 1% at Λ = 1 mm to about 8% at Λ = 10 mm. For the longer Λ and high precision studies, it would be necessary to consider the terms which were neglected in Eq. (35) and Eq. (40).
In an experiment, the fidelity may be affected by the spatial mode structure. These are very similar but not identical for the Y and Z polarized photons leaving the waveguide. For example, for 1250 nm photons, the overlap integral the electric fields for the two polarizations, (omitting the orthogonality due to polarization) is 0.97, when the two fields are normalized to unit self-overlap integrals. A simple way to nearly eliminate the effect of the spatial mode structure is to use a single mode optical fiber to produce identical spatial modes, albeit at the price of some coupling loss. (See Fig. 1.) Maintaining high efficiency throughout the optical path will require considerable care, including the use of antireflective coatings which reduces the need for reliance in posst selection by reducing the fraction of broken pairs. We also note that these losses do not affect fidelity, unless the contributions of background light or detector dark count rates become significant. In a similar way, polarization and frequency-dependent absorption can ameliorate the effect of an imbalance (i.e., deviation from unity) in the c 1/c −1 ratio discussed in Appendix B.
4. Concluding remarks
We have presented a proposal for a source of intrinsically-created polarization-entangled photons using type II parametric down conversion in a periodically-poled Rb:KTP waveguide. The new source’s simple optical design is expected to be more stable and easier to implement than previously demonstrated sources. The brightness and fidelity are expected to be comparable to the best existing sources.
The key feature of the new source is the simultaneous quasi-phase matching of photons using both orders m = ±1 of the periodically poled KTP waveguide A disadvantage of the scheme is that the available pump, signal, and idler wavelengths are highly constrained. However, we have shown that solutions are possible and even a common HeNe laser generating light at 632.8 nm may be used as a pump for certain geometries.
A. Spatial mode effect
After the introduction of Eq. (1), we noted that the effect of spatial modes disappears if the modes are identical. Here, we consider explicitly the effect of different spatial modes. In an ideally entangled Bell state of the type |YZ〉 + |ZY〉, we may perform the interchange Z ↔ Y with the state remaining invariant [31, 32]. (Other authors use |HV〉 + |VH〉 for our state |YZ〉 + |ZY〉.)
To avoid too much notational complexity, we will take β(ωs, ωi) ≈ β(ωi, ωs) in this Appendix. In analogy with Eq. (20), the norm is
using the normalization integral dr⃗|Uj(r⃗s, ωs)|2 = 1 for j = Y,Z. If we assume that the exchange integral is independent of frequency, then we have Thus, the net effect of the spatial mode structure on the fidelity is to make the exchange integral smaller by a factor of the spatial mode overlap integral in Eq. (24). For our waveguide, for λ = 625 nm, the spatial mode integral factor reduces the fidelity by a factor of 0.9738. The spatial modes are show for this case in Fig. 4 (bottom middle and bottom right). The modes are seen to be very similar, although not identical. The factor is only a weak function of the wave vector mismatch. For example, for Λ = 0.1 mm, 0.5 mm, and 1 mm, we obtain values of 0.8906, 0.9693, and 0.9697.As discussed in Sec. III, near Λ = 1 mm, the fidelity (omitting the spatial mode effect) can exceed 0.98. Hence, this may be the limiting factor in obtaining high fidelity. Manipulating the signal and idler beams after waveguide may be used to relieve this problem, in analogy to the temporal compensators which were established in the 1990’s. The simplest approach is to let the spatial modes enter a single mode fiber without polarization dependence.
B. Generation rates of two output channels
The coefficients c 1 and c −1 are proportional to matrix elements of the interaction Hamiltonian for parametric down conversion. This theory was developed for periodically poled waveguides by Fiorentino and coworkers [17] adapting an earlier development for parametric down conversion in periodically poled bulk crystals [11]. Indeed, the development of the present paper is anticipated to a certain extent by Ref. [11] in that they expand the position-dependent nonlinear coefficient d(x,z) as a Fourier series
which is Eq. (8) of Ref. [11]. (Our co-ordinate system in explained in Fig. 1(a).) They remark “the only term in Eq. (8) which will lead to a constructive interaction between the pump wave and the signal and idler is dn(x).” They then present a phase matching equation equivalent to our Eq. (6). Here, we consider more than one such term. Each yields the same form for the interaction matrix element which is given in Eq. (11) of Ref. [17] which is as written in the notation of the reference. Here, d is the effective nonlinear coefficient (2/π)dbulk [11], 𝒫p is the pump power, ε 0 is the electric constant, c is the speed of light, the n are indices of refraction, L is the crystal length, and A is the cross-sectional area of the waveguide, and the various U are the modes in the waveguide. In our case, we must remember that the n and d refer to the applicable polarization. We may write the ratio with where (ωs, ωi) is evaluated at .We estimate the dispersion of the nonlinear coefficients using Miller’s rule [33], namely
where δYZY is taken to be a constant and the χ are the linear susceptibilities, which are related to the index of refraction by . This permits us to estimate In the limit of degenerate parametric down conversion, i.e., inverse second harmonic generation, ωs = ωi, so c −1/c 1 = 1. This limit is obtained as Λ → ∞. As may be seen from the derivation in the text and Appendix C, the fidelity must be reduced by a factor of 2[(c –1/c 1)+(c 1/c −1)]−1 ≤ 1 assuming I ++ ≈ I −− using the symbols defined in Eq. (35).Numerical calculations for Λ = 0.1 mm, 0.5 mm, and 1 mm show that c −1/c 1 is 1.2084, 1.0365, and 1.0125 for the three cases, respectively. The deviation from unity is almost entirely due to the triple mode integral. The factors involving the index of refraction in Eq. (33) differ from unity by less than 10−4 for Λ ≥ 0.1 mm. Using the expression at the end of the previous paragraph, the fidelity needs to be reduced from that shown in Fig. 7 by a factor of 0.9823, 0.9994, and 0.9999, all of which are smaller than deviations from unity shown in the plot for the associated value of Λ. Hence, the approximation c 1 ≈ c −1 is justified.
C. Evaluation of direct and exchange integrals
The direct integral is given in Eq. (21) and the form of β is given by Eq. (3).
In an obvious notation, let There are large contributions where and to I ++, and large contributions when and to I −−, but the mixed terms are nowhere large, assuming that is always far from on the scale of oscillations of the sinc function. Formally, we require to neglect I +− = I −+. Equation (??) may be achieved in practice with periodically poled KTP.We may write I ++ as an integral over ξs and ξi as
For I −−, we interchange ωs and ωi,The exchange integral is given by
In a similar obvious notation similar to that above, let In this case, the terms J ++ and J −− may be neglected because the arguments to the two sinc functions are never simultaneously small. However, for J +− = J− + both arguments may be simultaneously small.If we take the pump bandwidth to be zero, Eq. (5) applies. Introducing δτ ± = τ ±1 s − τ ±1 i, the integrals in Eq. (37) and Eq. (38) reduce to
where Δτ ± = |δτ ±|. To obtain Eq. (42), we use the change of variables ξp = ξs + ξi and ξ = (ξs −ξi)/2 which has a unit Jacobian; also ξs = −ξi where the δ function of Eq. (5) is non-zero. Similarly, from Eq. (41), We may use Δτ ± instead of δτ ± because the sinc function is even.We may write
and J ≈ 2J +−. These expressions for I and J, combined with Eq. (24), lead to Eq. (25).Acknowledgments
Conversations with Eite Tiesinga are gratefully acknowledged. This work was supported in part by the Intelligence Advanced Research Projects Activity (IARPA) entangled photon source program.
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